Ab Initio Study of the Base-Catalyzed-Hydrolysis of Methyl Formate

by Pranata, J.

The intrinsic reaction coordinate pathway for the gas-phase, base-catalyzed hydrolysis of methyl formate has been determined using ab initio molecular orbital calculations at the MP2/6-31+G(d)//RHF/6-31+G(d) level of theory. Intermediate structures along the reaction pathway include an ion-dipole complex between the reactants, two conformationally distinct tetrahedral intermediates, and a hydrogen-bonded complex between the products.

Journal
Journal of Physical Chemistry
Volume
98
Issue
4
Year
1994
Start Page
1180-1184
URL
https://dx.doi.org/10.1021/j100055a023
ISBN/ISSN
0022-3654
DOI
10.1021/j100055a023